Scaling of phase matching of high-order harmonics into the multi-keV x-ray region at low ionization and large density-length products

ORAL

Abstract

In this work we investigate theoretically and experimentally how phase-matched high harmonic generation scales to multi-keV x-ray photon energies. We find that by using mid-infrared driving lasers of moderate intensity, this process presents an experimentally feasible and straightforward route for generating bright, fully coherent, beams even at multi-keV photon energies. We experimentally verify our predictions by demonstrating macroscopic phase-matched up-conversion of mid-IR laser light to water-window soft x-rays over extended distances in a high-density medium and moderate ionization levels. Finally, we show that the optimum phase matching pressures, absorption limited medium lengths, and macroscopic high harmonic yields scale very favorably with increasing driving laser wavelengths and x-ray photon energies, compensating for the decreasing single-atom signal strength at long driving wavelengths.

Authors

  • Tenio Popmintchev

    • JILA, University of Colorado at Boulder, NIST, NSF EUV ERC
  • Ming-Chang Chen

    • JILA, University of Colorado at Boulder, NIST, NSF EUV ERC
  • Alon Bahabad

    • JILA, University of Colorado at Boulder, NIST, NSF EUV ERC
  • Michael Gerrity

    • JILA, University of Colorado at Boulder, NIST, NSF EUV ERC
  • Paul Arpin

    • JILA, University of Colorado at Boulder, NIST, NSF EUV ERC
  • Matthew Seaberg

    • JILA, University of Colorado at Boulder, NIST, NSF EUV ERC
  • Richard Sandberg

    • JILA, University of Colorado at Boulder, NIST, NSF EUV ERC
  • Margaret Murnane

    • JILA, University of Colorado at Boulder, NIST, NSF EUV ERC
  • Henry Kapteyn

    • JILA, University of Colorado at Boulder, NIST, NSF EUV ERC
  • Pavel Sidorenko

    • Technion - Israel Institute of Technology
  • Oren Cohen

    • Technion - Israel Institute of Technology
  • Sterling Backus

    • Kapteyn-Murnane Laboratories Inc.
  • Xiaoshi Zhang

    • Kapteyn-Murnane Laboratories Inc.
  • Greg Taft

    • Kapteyn-Murnane Laboratories Inc.
  • Ivan Christov

    • Sofia University