A comparative study of dissociation and ionization of isoelectronic N$_{2}^{+ }$and CO$^{+}$ molecular ions in an ultrafast intense laser field.

POSTER

Abstract

The response of the molecular ion beams N$_{2}^{+ }$and CO$^{+}$ to intense (up to 5$\times $10$^{15}$ W/cm$^{2})$ ultrashort laser pulses (10 and 45 fs) at 790 nm wavelength is investigated. For this purpose, we employ a coincidence 3D momentum imaging method to separate all breakup channels and then obtain kinetic energy release spectra and angular distributions of each of the channels. In particular, we will make a direct comparison between N$_{2}^{+}$ and CO$^{+}$ fragmentation focusing on the similarities and differences of these two molecules that share similar electronic configurations. The relative branching ratios of all the relevant breakup channels will also be discussed.

*Supported by the Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy.

Authors

  • B. Gaire

    • J.R. Macdonald Laboratory, Department of Physics, Kansas State University
  • Nora G. Johnson

    • J.R. Macdonald Laboratory, Department of Physics, Kansas State University
  • J. McKenna

    • J.R. Macdonald Laboratory, Department of Physics, Kansas State University
  • A.M. Sayler

    • J.R. Macdonald Laboratory, Department of Physics, Kansas State University
  • E. Parke

    • J.R. Macdonald Laboratory, Department of Physics, Kansas State University
  • K.D. Carnes

    • J.R. Macdonald Laboratory, Department of Physics, Kansas State University
  • B.D. Esry

    • J.R. Macdonald Laboratory, Department of Physics, Kansas State University
  • I. Ben-Itzhak

    • J.R. Macdonald Laboratory, Department of Physics, Kansas State University