Ab Initio Electronic Dynamics of H$_{2}$ in Strong Attosecond Laser Field

POSTER

Abstract

Using Multi-Configuration Time-Dependent Hartree Fock with adaptive multiresolution methods and self-adaptive time propagation techniques with controlled accuracy we analyze ionization yields, electron spectra and high-harmonic radiation of a hydrogen molecule in an attosecond strong laser pulse. We follow single- and two-electron dynamics of the process of ionization during a single field cycle, including rescattering imaging of a molecular orbital and the scattering production of harmonics.

*Work sponsored by the Office of Fusion Energy Sciences and the Office of Basic Energy Sciences of U.S. DOE under contract No. DEACO5-00OR22725 with UT Battelle, LLC.

Authors

  • P.S. Krstic

    • Physics Division, ORNL
    • ORNL
  • R. J. Harrison

    • CSMD, ORNL