Three-Step Model for High-Harmonic Generation in Many-Electron Systems

ORAL

Abstract

The three-step model (TSM) of high-harmonic generation (HHG) is generalized to atomic and molecular many-electron systems. Using many-body perturbation theory, corrections to the standard TSM due to exchange and electron--electron correlations are derived. It is shown that canonical Hartree-Fock orbitals represent the most appropriate set of one-electron states for calculating the HHG spectrum. To zeroth order in many-body perturbation theory, a HHG experiment allows direct access in general to a combination of occupied Hartree-Fock orbitals rather than to the highest occupied molecular orbital by itself.

*This work was supported in part by the Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy, under Contract No. W-31-109-ENG-38. Partial support by AFOSR under grant FA9550-04-1-0011 is gratefully acknowledged.

Authors

  • Robin Santra

    • Argonne National Laboratory, Argonne, IL 60439, USA
    • Argonne National Laboratory, Argonne, IL 60439
    • Argonne National Laboratory, Argonne, Illinois 60439, USA
  • Ariel Gordon

    • Research Laboratory of Electronics, Massachusetts Institute of Technology, 77 Massachusetts Ave., Cambridge, MA 02139