Exploring the parameter space for ionization and dissociation of H$_{2}^{+}$ in an intense laser pulse

POSTER

Abstract

We explore the dissociation and ionization of H$_{2}^{+}$ ions aligned with a 790~nm laser field of peak intensity in the range 1.0$\times $10$^{13}$ to 7.0$\times $10$^{14}$~W/cm$ ^{2} $. Calculated dissociation and ionization probabilities are reported for different initial vibrational states and for the initial state averaged over the Franck-Condon distribution. The dependence on the carrier-envelope phase difference for different initial states and for pulse durations from 5 to 30~fs FWHM is presented. These results --- from direct solution of the time-dependent Schr\"odinger equation --- are compared with solutions in the Born-Oppenheimer representation with two-channels for low peak laser intensities.

*This work wassupported by the Chemical Sciences, Geosciences,and Biosciences Division, Office of Basic Energy Sciences, Office of Science,U.S.Department of Energy.

Authors

  • Vladimir Roudnev

    • J.R. Macdonald laboratory, Department of Physics, Kansas State University
  • B.D. Esry

    • J.R. Macdonald Laboratory, Department of Physics, Kansas State University
    • Physics Department, Kansas State University
    • J. R. Macdonald Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506